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Electron-doped cuprates have mainly been studied in the T′ structure because chemical electron doping tends to destabilize the T phase. Here, we realize electron-doped T-phase La2CuO4 (LCO) monolayers using polar discontinuity at oxide interfaces. Charging-free LCO/LAO/LSCO heterostructures were fabricated by pulsed laser deposition and studied by ARPES. The LCO monolayer exhibits a clear Fermi surface, unlike insulating bulk-like LCO, indicating successful electron doping. Tight-binding analysis shows that the electron doping level increases with LAO buffer-layer thickness, consistent with charge redistribution driven by polar discontinuity. However, thicker LAO layers also degrade the ARPES spectral quality, suggesting additional compensation mechanisms such as surface reconstruction. These results demonstrate polar discontinuity as a promising route to electron-doped T-phase cuprates.
목차
Abstract 1. 서론 2. 실험 방법 3. 결과 및 논의 4. 결론 ACKNOWLEDGMENT REFERENCES